Must have N64 Games (that aren't on Wii VC)

[YoshiM]

This bit always confused me. Is LoD a remake of CV64, a sequel, or a prequel? From what I've seen it sort of looks like a remake with a different story line.

Tempest

I've never played it but with the different storyline (takes place 8 years before CV64), the addition of new characters and weapons-you could almost count it as a prequel running on the same engine.

As for suggestions, people pretty much hit the biggies. Here's some I can recommend:

Space Station Silicon Valley (though it can't be played with the memory expansion installed)
Star Wars Rogue Squadron
New Tetris
Star Wars Episode 1: Racer (use two controllers to pilot your pod racer)
Body Harvest
Excitebike 64
F-Zero X